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Ultrafast IR and raman spectroscopy 2001 fayer

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Ultrafast IR and raman spectroscopy 2001 fayer

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Xem thêm: Ultrafast IR and raman spectroscopy 2001 fayer , I. COHERENT ANTI-STOKES RAMAN SPECTROSCOPY OF SIMPLE LIQUIDS, II. TIME-RESOLVED IR SPECTROSCOPY OF STRONGLY ASSOCIATED LIQUIDS, Ethanol Oligomers in Solution: Spectral Holes and Vibrational Lifetime Shortening, H-Bonded Dimers: Librational Substructure of the OH Band of Proton Donors, E. Investigations of Isotopic Water Mixtures, A. The Dynamics of Reaction Intermediates — Vibrational Relaxation and Molecular Morphology Change, B. The Activation Barrier — The Bond-Breaking Step, A. The Reaction Intermediates — Solvation-Partitioned Pathways and Intersystem Crossing, B. The Reaction Barrier — Solvent Molecule Rearrangement, C. The Reaction Mechanism — Resolving a Convolved Chemical Reaction, A. Clarification of the Reaction Pathway, B. The Nature of the Reaction Barrier — Atom Transfer, E. Vibrational Coherent Control with Chirped Picosecond Infrared Excitation, F. Ultraviolet Photochemistry: Self-Association Reactions of Mn(CO)3CpR Species and [CpFe(CO)2]2 in Solution, G. Primary Electron Transfer Dynamics of Dye-Sensitized Semiconductor Solar Cell Devices, IV. CONCLUSIONS AND FUTURE DIRECTIONS, A. Vibrational Energy Relaxation and Vibrational Friction, B. The Instantaneous Vibrational Friction and the Instantaneous Normal Modes of the Solvent, III. HOW COLLECTIVE IS VIBRATIONAL ENERGY RELAXATION?, IV. HOW DOES DIELECTRIC FRICTION EFFECT VIBRATIONAL ENERGY RELAXATION?, V. VIBRATIONAL ENERGY RELAXATION AT HIGH FREQUENCIES, A. Vibrational Spectrum of Orientationally Constrained CO, A. Laser Photolysis: A Sledgehammer or a Scalpel?, B. Evidence for a Ligand Docking Site in the Heme Pockets of Mb and Hb, C. Orientation of Bound and ‘‘Docked’’ CO, E. Origin of the Barrier to CO Rebinding, A. The Vibrational Echo Method, III. VIBRATIONAL ECHO STUDIES OF DYNAMICS IN LIQUIDS AND CLASSES, A. Vibrational Echo Spectroscopy Theory, C. Experimental Demonstrations of VES, A. Vibrational Echo Results and Dephasing Mechanisms, B. Coupling of Protein Fluctuations to the CO Ligand at the Active Site, III. SPECTRAL DIFFUSION OF VIBRATIONAL TRANSITIONS, A. Theory of Vibrational Third-Order Nonlinear Spectroscopy, D. The Three-Pulse Photon Echo Experiment, E. Spectral Diffusion of Small Molecules in Water, F. Spectral Diffusion of Vibrational Probes in Enzyme-Binding Pockets, A. An Excitonic Model for the Amide I Band, C. Two-Dimensional IR Spectroscopy on the Amide I Band, D. Spectral Diffusion of the Amide I Band, E. 2D-IR Spectroscopy Using Semi-Impulsive Methods, II. THREE-PULSE MULTIDIMENSIONAL FEMTOSECOND OPTICAL SPECTROSCOPIES, IV. VIBRATIONAL EXCITONS IN CYCLIC PENTAPEPTIDE, A. Absolute Value of the 2D Signal, B. Real and Imaginary Parts of the 2D Signal, A. One-Dimensional Measurements: Raman Line Shape and Free Induction Decays, B. A Two-Dimensional Measurement: The Raman Echo, III. IMPLEMENTING COHERENT RAMAN EXPERIMENTS, C. Special Problems of Seventh-Order Spectroscopy, A. Concentration Fluctuations in CH3I:CDCl3, B. Density Fluctuations in Acetonitrile, D. A Viscoelastic Theory of Vibrational Dephasing, E. Solvent-Assisted IVR in Ethanol, A. General: Nonresonant Nonlinear Optical Response, C. Cascaded Fifth-Order Electronically Nonresonant Scattering, B. Intramolecular Vibrations in Carbon Tetrachloride, B. Intermolecular Motions in CS2, C. Intramolecular Vibrations in Carbon Tetrachloride and Chloroform, V. SYMMETRIC-TOP LIQUIDS: ORIENTATIONAL DIFFUSION, VI. SYMMETRIC-TOP LIQUIDS: INTERMOLECULAR SPECTRA, IV. SUMMARY AND FUTURE PROSPECTS, B. Force Correlation Function Approach, B. Pseudo-vibrational Cascade in Nitromethane, C. Dynamics of Doorway Vibrations, E. Fermi Resonance and Overtones, G. Spectral Evolution in Associated Liquids, II. COULOMBIC FORCE EFFECTS ON VET, III. SOLUTE INTRAMOLECULAR EFFECTS ON VET, B. Gas Phase Vibrational Dynamics, IV. THEORY OF T1 IN SUPERCRITICAL FLUIDS, V. COMPARISON OF THEORY AND EXPERIMENT, II. GENERAL THEORY OF VIBRATIONAL ENERGY RELAXATION, III. I2 IN LIQUID AND SUPERCRITICAL XENON, V. W(CO)6 IN SUPERCRITICAL ETHANE

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Mục lục

  • DK1709_FM.PDF

    • Ultrafast Infrared and Raman Spectroscopy

      • PRACTICAL SPECTROSCOPY, A SERIES

      • Preface

      • Table of Contents

      • Contributors

      • DK1709_CH01.PDF

        • Ultrafast Infrared and Raman Spectroscopy

          • Table of Contents

          • Chapter 01: Ultrafast Coherent Raman and Infrared Spectroscopy of Liquid Systems

            • I. COHERENT ANTI-STOKES RAMAN SPECTROSCOPY OF SIMPLE LIQUIDS

              • A. Introduction

              • B. General Considerations

              • C. Experimental Aspects

              • D. Results and Discussion

                • 1. Reorientational Motion of Liquid Molecules in Time-Domain CARS

                • 2. Time Scale of the Dominant Dephasing Mechanism

                • 3. Measurements of Specific Dephasing Channels

                • 4. Resonant Vibrational Dephasing

                • 5. Vibrational Dephasing in the Intermediate Case

                • II. TIME-RESOLVED IR SPECTROSCOPY OF STRONGLY ASSOCIATED LIQUIDS

                  • A. Introduction

                  • B. General Considerations

                  • C. Experimental Aspects

                  • D. Alcohols in Solutions

                    • 1. Monomers in an Apolar Solution

                    • 2. Ethanol Oligomers in Solution: Spectral Holes and Vibrational Lifetime Shortening

                    • 3. Fully Associated Ethanol in Isotopic Mixtures

                      • a. Diluted Isotopic Mixture (1 vol% protonated ethanol)

                      • b. Concentrated Isotopic Mixture (50 vol% protonated ethanol)

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